Well, it was worth a try...
If you set the center to large, the crossover will be irrelevent as there will be no bass management applied to that speaker. The Cinema i's -3dB point is 80Hz, so I wouldn't go below that crossover point. In fact, I'd probably try 100Hz as a crossover for the Cinema i. After all, dialog is going to be a
long way up from the crossover point, so we're mainly just trying to make sure that the speaker isn't being asked to do things it's not capable of.